本文综述了利用高温蒸发物理气相沉积(HT-ePVD)方法在制备离子组分精确的低温度功能钙钛矿材料方面的进展。结合高通量材料库的合成和筛选技术，该方法能快速确定结构与功能之间的关系。通过调控A位和/或B位阳离子替代，以及阴离子替代，可以轻松探索材料的性能调谐，适用于各种钙钛矿系统，对多种技术有潜在应用价值。
摘要：
The development of functional perovskites for future technologies can be achieved though the combinatorial synthetic method of evaporative physical vapour deposition (HT-ePVD) which provides a direct low temperature route to anion stoichiometric materials. When combined with the ability to control and vary precisely the composition of thin film libraries of materials, high-throughput methods of screening and characterisation provides a rapid experimental determination of the structure/function relationship. This review of the use of HT-ePVD shows that controlled cationic substitutions in A and/or B sites can easily be explored, as can the effect of anionic substitution. This is exemplified in using this approach for a wide range of perovskite systems, where the tuning of the functional properties through cation substitution has application in a broad range of technologies.
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