Lecture - 3 PDF
Lecture - 3 PDF
SASTRA University
Table of Contents
1
BREEDING
.......................................................................................................................................
3
1.1
BREEDING
RATIO
........................................................................................................................................
4
1.2
BREEDING
GAIN
..........................................................................................................................................
4
1.3
DOUBLING
TIME
(DT)
...............................................................................................................................
5
2
REFERENES/ADDITIONAL
READING
.....................................................................................
7
In this lecture, we shall discuss about the calculation of breeding ratio and doubling
time
1 Breeding
Breeding in nuclear reactors refers to the process in which significantly amount of
fertile materials are converted to fissile materials by nuclear transmutation. This
requires the fertile isotope to have large cross section for neutron capture. Since the
main purpose of a nuclear reactor is to produce electricity, breeding is considered as
an off-shoot of excess neutrons produced during fission above the ones required for
sustenance of chain reaction.
The possibility of breeding in a nuclear reactor, taking into account of the type of
fissile material used, depends on the number of neutrons produced for every neutron
absorbed in the fuel. This is denoted by reproduction factor ‘η’. This is related to the
cross sections as follows:
σf
η= ν (1)
σa
The probability of breeding is enhanced when the value of ‘η’ exceeds two by a large
fraction. For example, the value of ‘η’ for U-235, Pu-239 and U-233 when
bombarded by thermal neutrons is 2.07, 2.11 and 2.30 respectively. Breeding with
thermal neutrons using U-235 and Pu-239 fuels is virtually impossible due to neutron
absorption in structural materials and moderator. However, with U-233 fuel, it is
possible to achieve breeding using thermal neutrons.
The scenario is different for the case of bombardment with fast neutron. The value of
‘η’ for U-235, Pu-239 and U-233 when bombarded by fast neutrons is 2.3, 2.7 and
2.45 respectively. Hence, breeding is possible with all the above fissile nuclei due to
bombardment with fast neutron.
Conversion ratio is a widely used term to denote the ability of a reactor to convert
fertile to fissile material. Conversion ratio is defined as the ratio of number of fissile
nuclei produced to the number of fissile nuclei consumed.
When a reactor is operated without any fertile material, the conversion ratio is zero. In
this case, the reactor is referred to as ‘burner’ as it burns all the fuel without
producing any fissile material.
It may be recalled that the uranium fuelled thermal reactors either use natural uranium
or enriched uranium. In both these cases, isotopic abundance of U-238, a fertile
material, is very high. It is possible to achieve a higher conversion ratio by facilitating
higher neutron capture in U-238 relative to neutron absorption in U-235. This must be
carried out without the loss of criticality. To ensure that sufficient neutrons are
available for chain reaction, the neutron losses in structural elements and moderator
must be reduced. Also, the use of moderators like heavy water and carbon require
more collisions for neutron thermalization and hence require larger core. This
improves the contact between neutron and U-238 contact, thereby improving the
conversion ratio.
The breeding ratio is maximum when the leakage of neutrons (l) is zero. This is called
maximum breeding ratio (BRmax) and is also called Breeding Potential of the fuel.
Please note that in Eq. (3), ‘ε’ the fast fission factor is taken as unity as most of the
breeders are fast breeders. The reproduction factor is to be calculated for Pu-239, the
predominant fissile isotope in fast reactors.
BG = BR – 1 (3)
This represents the extra fissile material produced for every atom of fuel (fissile
isotope) consumed.
BR = η239-1-l (4)
⎛ σ f ⎞
CR= BR = ⎜⎜ ν ⎟⎟ − 1 − l (5)
⎝ σ a ⎠ 239
Example -1: Determine Breeding Ratio for Pu-239 fuelled fast reactor. Take ν =
2.975; σ f = 1.850; σ a = 2.11 and l = 0.405.
1.85
Using Eq. (5), BR = ⎛⎜ ⎞
2.975 ⎟ − 1 − 0.405
⎝ 2.11 ⎠
BR = 1.203
The reactor power per unit mass of fuel (P’) may be related to the number of fuel
nuclei per unit mass of the fuel (Nf) as
P’=EfNfφ-σf (6)
Power per unit mass of fuel (W/kg)= Energy released per fission (J) * Number
fissions per unit time per unit mass of fuel (s-1kg-1)
The number of fissions per unit time per unit mass of fuel represents the rate of
consumption of a unit mass of fuel.
Therefore, If MF is the mass of fuel loaded, then the rate of consumption (RC) of fuel
of mass MF is given by
If ‘BR’ is the Breeding Ratio, then the rate of production (RP) of fissile mass is given
by
RP = BR*MFNfφ σa (atoms/s)
−
(8)
DT*Rnet=MFNf (10)
Therefore,
MFN f MFN f 1
DT = = =
Rnet (BR − 1)M F N f φ −
σa (BR − 1)φ −σ a
(11)
Recall, P’=EfNfφ-σf
N f Efσ f
DT = (13)
(BR − 1)σ a P '
Now let’s discuss the factors that influence Doubling Time.
(i) Breeding Ratio: Higher the Breeding Ratio, greater is the amount of fissile material
produced. Hence, the time required for doubling the mass is reduced at higher
Breeding Ratios. We have seen earlier that Breeding Ratio depends on the
reproduction factor η, which inturn is influenced by absorption cross section,
fission cross sections and ‘ν'. As the cross sections are functions of neutron
energies, appropriate choice of neutron energy and steps to minimize neutron
leakage will result in increased Breeding Ratio (BR).
(ii) Power per unit mass of the fuel: When this quantity is high, the average neutron
flux is also high among other variables. As evident from Eq. (11), with increased
neutron flux, the Doubling Time is reduced. Hence the Doubling time decreases
with increased reactor Power per unit mass of the fuel.
Example – 4: Determine the doubling time of a Pu-239 fast breeder reactor. The
reactor is operated at 400 MW/tonne Pu-239 with a Breeding Ratio of 1.2. The
absorption and fission cross section are 2.16 and 1.81 b respectively. The number
of Pu-239 per unit mass is 2.52x1021 (atoms/g).
σa = 2.16 b; σf = 1.81 b
2 Referenes/Additional Reading
1. Nuclear Energy: An Introduction to the Concepts, Systems, and Applications of
Nuclear Processes, 5/e, R.L. Murray, Butterworth Heinemann, 2000 (Chapter 13).