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Poster Igac 2021

1) The document evaluates the direct and indirect effects of vehicular emissions on air quality and meteorology in Southeast Brazil using an emissions inventory model and air quality simulation model. 2) It finds that simulating parameters like NO2, NO, and O3 concentrations align with observations when including aerosol effects, though PM2.5 correlations were lower. 3) Including aerosol effects reduced surface downward shortwave radiation by around 2%, consistent with other studies, showing the meteorological impacts of aerosols.
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0% found this document useful (0 votes)
36 views1 page

Poster Igac 2021

1) The document evaluates the direct and indirect effects of vehicular emissions on air quality and meteorology in Southeast Brazil using an emissions inventory model and air quality simulation model. 2) It finds that simulating parameters like NO2, NO, and O3 concentrations align with observations when including aerosol effects, though PM2.5 correlations were lower. 3) Including aerosol effects reduced surface downward shortwave radiation by around 2%, consistent with other studies, showing the meteorological impacts of aerosols.
Copyright
© © All Rights Reserved
We take content rights seriously. If you suspect this is your content, claim it here.
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Download as PDF, TXT or read online on Scribd
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Direct and indirect effects of aerosols on meteorology and air pollutant concentrations

during dry and wet periods on Southeast Brazil


Sergio Ibarra-Espinosa 1, , Gyrlene Aparecida Mendes da 2
Silva , Amanda Rehbein 1, , Angel Vara-Vela 3, , Edmilson Dias de
Freitas 1,
1 Departamento de Ciências Atmosféricas, Instituto de Astronomia, Geofísica e Ciências Atmosféricas, Universidade de São Paulo; São Paulo-SP, Brazil; 2 Instituto do Mar,

Universidade Federal de São Paulo; Santos-SP, Brazil; 3 Federal University of Technology - Parana; Londrina, Brazil

Introduction
Conclusion
Air pollution is generated by complex interactions between emissions and
meteorology. Air pollutants disperse in the atmosphere, but they suffer In this study we evaluated the effects of vehicular emissions on air quality.
transformations generating secondary pollutants such as aerosols and The simulated parameters align with observations in most of cases, with
gases such as ozone (Kong et al. 2015). Furthermore, aerosols have effects correlations above 0.8 and 0.9, but P M correlations were about 0.5 (not 2.5

on meteorology, direct with absorbing and scattering solar radiation, and shown). There is a positive bias for N O and negative for N O , suggesting 2

indirect by increasing the cloud concentration numbers affecting that emission factors for vehicles needs to be improved. (2016) aerosols
precipitation (Penner et al. 2001). The most important source of air reduce O on 2%, similar to our study.
3

pollution in South East Brazil are vehicles (CETESB 2020). Then, in this
study, we evaluated the effects of vehicular emissions on air quality and G.A.M. da Silva thanks CNPq, Nº. 426221/2016-8. E.D.F. FAPESP Grants Nº. 2015/03804-9 and 2016/18438-0; A.R. 2016/10557-0; and S.I.E 2021/07136-1.

meteorology on South East Brazil using a bottom-up emissions inventory.


References
Objectives Carter, William PL. 2015. “Development of a Database for Chemical
Mechanism Assignments for Volatile Organic Emissions.” Journal of the
1. Elaborate vehicular emissions inventory. Air & Waste Management Association 65 (10): 1171–84.
Figure 1: Emissions PM2.5 08:00-09:00 [g/h/km²]
2. Simulate air pollutant concentrations with and without activating CETESB. 2020. “Emissões Veiculares No Estado de são Paulo 2019.”
aerosol feedbacks. Grell, Georg A, Steven E Peckham, Rainer Schmitz, Stuart A McKeen,
3. Statistical analysis. Gregory Frost, William C Skamarock, and Brian Eder. 2005. “Fully
Coupled ‘Online’ Chemistry Within the WRF Model.” Atmospheric
Environment 39 (37): 6957–75.
Methods Ibarra-Espinosa, S., R. Ynoue, S. O’Sullivan, E. Pebesma, M. D. F.
Andrade, and M. Osses. 2018. “VEIN V0.2.2: An r Package for Bottom–up
To estimate the vehicular emissions we used the VEIN model (S. Ibarra- Vehicular Emissions Inventories.” Geoscientific Model Development 11 (6):
Espinosa et al. 2018), which already incorporates brazilian emissions 2209–29. https://doi.org/10.5194/gmd-11-2209-2018.
factors (CETESB 2020) adjusted by real-world tunnel measurements Ibarra-Espinosa, Sergio, Rita Yuri Ynoue, Karl Ropkins, Xuelei Zhang, and
(Nogueira et al. 2021). Vehicular activity was obtained from 104 million Edmilson Dias de Freitas. 2020. “High Spatial and Temporal Resolution
GPS registries from smart-devices inside vehicles in circulation (Sergio Vehicular Emissions in South-East Brazil with Traffic Data from Real-Time
Ibarra-Espinosa et al. 2019). Furthermore, the vehicular activity was GPS and Travel Demand Models.” Atmospheric Environment 222: 117136.
adjusted by fuel consumption on our region of study as shown by Sergio Figure 2: Difference in downward short wave flux at ground surface (W/m²) after activating aerosol effects
Ibarra-Espinosa, Sergio, Rita Ynoue, Mariana Giannotti, Karl Ropkins, and
Ibarra-Espinosa et al. (2020). Emissions estimation were aggregated in Edmilson Dias de Freitas. 2019. “Generating Traffic Flow and Speed
RADM2/MADE/SORGAM groups applying the methodology of . Carter Regional Model Data Using Internet GPS Vehicle Records.” MethodsX 0
(2015). The period of study dry was 2014-10-05 to 2014-10-10 and wet (March).
2014-10-31 to 2014-11-05. Air pollutant concentrations were obtained Kong, Xin, Renate Forkel, Ranjeet S Sokhi, Peter Suppan, Alexander
using the model WRF-Chem (Grell et al. 2005). Baklanov, Michael Gauss, Dominik Brunner, et al. 2015. “Analysis of
Meteorology–Chemistry Interactions During Air Pollution Episodes Using
Online Coupled Models Within AQMEII Phase-2.” Atmospheric
Results Environment 115: 527–40.
Nogueira, Thiago, Leonardo Yoshiaki Kamigauti, Guilherme Martins
We corroborated the dry and wet periods using surface observational data Pereira, Mario E Gavidia-Calderón, Sergio Ibarra-Espinosa, Guilherme
from CETESB and national institute of meteorology INMET. The Librete de Oliveira, Regina Maura de Miranda, Pérola de Castro
vehicular emissionsare higher than official estimates, because of the Vasconcellos, Edmilson Dias de Freitas, and Maria de Fatima Andrade.
emission factors adjusted by tunnel measurements, and by the adjustment Figure 3: Difference in precipitation (mm/h) after activating aerosol effects 2021. “Evolution of Vehicle Emission Factors in a Megacity Affected by
of activity with real fuel automotive consumption. The gridded emissions Extensive Biofuel Use: Results of Tunnel Measurements in São Paulo,
maps for P M 2.5 is shown on Figure 1 which includes exhaust and Brazil.” Environmental Science & Technology 55 (10): 6677–87.
ressuspension emissions. Figure 2 shows that the biggest effect of aerosols Penner, Joyce E, MO Andreae, H Annegarn, L Barrie, J Feichter, D Hegg,
is found during dry period, in São Paulo center. On Figure 3 we can see A Jayaraman, et al. 2001. “Aerosols, Their Direct and Indirect Effects.” In
the enhancement of precipitation during wet period, because the average Climate Change 2001: The Scientific Basis. Contribution of Working Group
value for the whole domain is 0.02, which corroborates more i to the Third Assessment Report of the Intergovernmental Panel on Climate
precipitation. The enhancement of precipitation is produced in center and Change, 289–348. Cambridge University Press.
west part of domain. However, we can see less precipitation in a red strip Vara-Vela, Angel, Maria F Andrade, Prashant Kumar, Rita Y Ynoue, and
center to domain to Santos, suggesting association with sea-breeze. Lastly, Angel G Munoz. 2016. “Impact of Vehicular Emissions on the Formation of
the Figure 4 shows the percentage change of O after activating aerosol
3
Fine Particles in the Sao Paulo Metropolitan Area: A Numerical Study with
effects during dry period. The max percentage change was 1.5% at the WRF-Chem Model.” Atmospheric Chemistry and Physics 16 (2): 777–
CETESB stations. Furthermore, the average percentage of O was -0.14%
3
97.
for the whole domain.
Figure 4: Difference in surface O3 (%) after activating aerosol effects for dry period

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